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How Many Pokémon Can You Get Without Evolving or Breeding in Pokémon LeafGreen?

The player can get up to 171 species total in LeafGreen without trading, as described here. Without evolving or breeding any Pokémon, and only collecting evolutionary stages that the player can get in the wild, as a gift or purchase, or from an in-game trade, the player can get up to 100 species in the Kanto Pokédex and 122 in the National Pokédex. The Pokémon unavailable without evolving or breeding are as follows:

Kanto Pokédex

Starter Evolutions (2) - 2 total
The starters are only available in their base evolutionary stages, leaving their evolutions inaccessible.
Stone Evolutions (11) - 13 total
Raichu, Nidoqueen, Nidoking, Clefable, Ninetales, Wigglytuff, Poliwrath, Victreebel, Exeggutor, Starmie, and Eevee's evolutions are inaccessible.
Two Eevee evolutions (2) - 15 total
Without the ability to breed, the other two evolutions of Eevee are not accessible.
One of Hitmonlee/Hitmonchan (1) - 16 total
Without the ability to breed, the other of Hitmonlee or Hitmonchan is not accessible.
Fossils (1) - 17 total
The Fossils can only be revived into their base evolutionary stages, leaving their evolutions inaccessible.
Other (8) - 25 total
Butterfree, Beedrill, Pidgeot, Dodrio, Weezing, Rhydon, Seadra, and Dragonite are inaccessible.

National Pokédex

Evolving from Kanto Pokémon (2) - 27 total
Crobat and Blissey evolve from Kanto Pokémon and are inaccessible.
Breeding from Kanto Pokémon (7) - 34 total
Pichu, Cleffa, Igglybuff, Tyrogue, Smoochum, and Magby must be bred from Kanto Pokémon and are inaccessible. Hitmontop evolves from Tyrogue and is also inaccessible.
Breeding from National Pokédex Pokémon (2) - 36 total
Wynaut must be bred from Wobbuffet, and Azurill from Marill or Azumarill, and is inaccessible.
Other (13) - 49 total
Furret, Ledian, Ariados, Togetic, Xatu, Azumarill, Skiploom, Jumpluff, Piloswine, Octillery, Donphan, Pupitar, and Tyranitar are inaccessible.

With access to the Ho-Oh, Lugia, and Deoxys that can be obtained in the Switch rereleases of LeafGreen, the player can get a total of 125 Pokémon.

Professor Oak(-ish) Challenge Notes

This just contains a list of areas you can find each Pokémon, ordered as though you are playing a Professor Oak challenge and therefore need to obtain every Pokémon as early as possible.

Pre-Badge 1 (Brock) - 10 Total Pokémon

Badge 1 through Badge 2 (Misty) - 27 Total Pokémon

Badge 2 through Badge 3 (Koga) - 70 Total Pokémon

Badge 3 through Badge 4 (Blaine) - 85 Total Pokémon

Badge 4 through Badge 5 (Erika) - 89 Total Pokémon

Badge 5 through Badge 6 (Sabrina) - 94 Total Pokémon

Badge 6 through Badge 8 - 96 Total Pokémon

Badge 8 through Elite Four - 98 Total Pokémon

Post-Elite Four - 100 Total Pokémon

Post-Elite Four - National Pokédex - 122 Total Pokémon

All National Pokédex Pokémon are only available after defeating the Elite Four.

If you are able to obtain Ho-Oh, Lugia, and Deoxys, the total for this section is 125.